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3 New Materials At this point it would be useful to discuss the possible band gaps necessary for the as yet unknown materials to be used in an eﬃcient solar photoelectrolysis device. The band gap values should be used as a guide for researchers’ eﬀorts on the discovery and optimization of these materials. 21 Calculations of theoretical eﬃciencies all hinge on assumptions of eﬃciency losses, which are primarily the overpotential losses for the hydrogen and oxygen half reactions. The eﬃciency loss estimates are typically based on the losses observed in electrolysis cells.
Zunger, N. H. Perry, Y. Tang, M. Grayson, T. O. Mason, J. S. Bettinger, Y. Shi and M. F. Toney, Phys. Rev. , 2011, 84, 205207. 43. B. D. James, G. N. Baum, J. Perez, K. N. pdf (December 2009). 14/10/2013 09:37:11. 1 Introduction This chapter examines a range of electrochemical, optical and other experimental methods that can be used to obtain information about the kinetics and mechanisms of electrode reactions driven by the capture of photogenerated minority carriers at the interface between an electrolyte and an illuminated semiconductor electrode.
Transparent substrates could be used in this case, since back illumination of both gas-evolving electrodes would eliminate all of the backscattering of light from bubbles that prevents it from reaching the photoelectrodes. The result is that the number of possible material systems is broadened and cheaper or more abundant materials may be utilized. 1 summarizes some of the advantages and disadvantages of the diﬀerent photoelectrolysis conﬁgurations discussed above. Systems that contain buried junctions, where charge separation is remote from the electrolyte, are really solid state solar cells in series with metal electrodes, and they are not considered here since they are essentially equivalent to hooking up photovoltaic cells to an electrolysis cell, albeit without the wires.